Differently Prepared PbO2/Graphitic Carbon Nitride Composites for Efficient Electrochemical Removal of Reactive Black 5 Dye

In this paper, electrochemical degradation of Reactive Black 5 (RB5) textile azo dye was examined in regard to different synthesis procedures for making PbO2–graphitic carbon nitride (g-C3N4) electrode. The reaction of with ClO− in the presence of different surfactants, i.e., cetyltrimethylammonium...

Teljes leírás

Elmentve itt :
Bibliográfiai részletek
Szerzők: Marković Aleksandar
Savić Slađana
Kukuruzar Andrej
Kónya Zoltán
Manojlović Dragan
Ognjanović Miloš
Stanković Dalibor M.
Dokumentumtípus: Cikk
Megjelent: 2023
Sorozat:CATALYSTS 13 No. 2
Tárgyszavak:
doi:10.3390/catal13020328

mtmt:33612005
Online Access:http://publicatio.bibl.u-szeged.hu/34059
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245 1 0 |a Differently Prepared PbO2/Graphitic Carbon Nitride Composites for Efficient Electrochemical Removal of Reactive Black 5 Dye  |h [elektronikus dokumentum] /  |c  Marković Aleksandar 
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490 0 |a CATALYSTS  |v 13 No. 2 
520 3 |a In this paper, electrochemical degradation of Reactive Black 5 (RB5) textile azo dye was examined in regard to different synthesis procedures for making PbO2–graphitic carbon nitride (g-C3N4) electrode. The reaction of with ClO− in the presence of different surfactants, i.e., cetyltrimethylammonium bromide (CTAB) and tetrabutylammonium phosphate (TBAP), under conventional conditions, resulted in the formation of PbO2 with varying morphology. The obtained materials were combined with g-C3N4 for the preparation of the final composite materials, which were then characterized morphologically and electrochemically. After optimizing the degradation method, it was shown that an anode comprising a steel electrode coated with the composite of PbO2 synthesized using CTAB as template and g-C3N4, and using 0.15 M Na2SO4 as the supporting electrolyte, gave the best performance for RB5 dye removal from a 35 mg/L solution. The treatment duration was 60 min, applying a current of 0.17 A (electrode surface 4 cm2, current density of 42.5 mA/cm2), while the initial pH of the testing solution was 2. The reusability and longevity of the electrode surface (which showed no significant change in activity throughout the study) may suggest that this approach is a promising candidate for wastewater treatment and pollutant removal. 
650 4 |a Kémiai tudományok 
700 0 1 |a Savić Slađana  |e aut 
700 0 1 |a Kukuruzar Andrej  |e aut 
700 0 1 |a Kónya Zoltán  |e aut 
700 0 1 |a Manojlović Dragan  |e aut 
700 0 1 |a Ognjanović Miloš  |e aut 
700 0 1 |a Stanković Dalibor M.  |e aut 
856 4 0 |u http://publicatio.bibl.u-szeged.hu/34059/1/catalysts-13-00328-v2.pdf  |z Dokumentum-elérés