Laser-induced inner-shell excitations through direct electron re-collision versus indirect collision

The dynamics and the decay processes of inner-shell excited atoms are of great interest in physics, chemistry, biology, and technology. The highly excited state decays very quickly through different channels, both radiative and non-radiative. It is therefore a long-standing goal to study such dynami...

Teljes leírás

Elmentve itt :
Bibliográfiai részletek
Szerzők: Deng Yunpei
Zeng Zhinan
Komm Pavel
Zheng Yinghui
Helml Wolfram
Xie Xinhua
Filus Zoltán
Dumergue Mathieu
Flender Roland
Kurucz Máté
Haizer Ludovit
Kiss Bálint
Kahaly Subhendu
Li Ruxin
Marcus Gilad
Dokumentumtípus: Cikk
Megjelent: 2020
Sorozat:OPTICS EXPRESS 28 No. 16
Tárgyszavak:
doi:10.1364/OE.395927

mtmt:31733452
Online Access:http://publicatio.bibl.u-szeged.hu/26944
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490 0 |a OPTICS EXPRESS  |v 28 No. 16 
520 3 |a The dynamics and the decay processes of inner-shell excited atoms are of great interest in physics, chemistry, biology, and technology. The highly excited state decays very quickly through different channels, both radiative and non-radiative. It is therefore a long-standing goal to study such dynamics directly in the time domain. Using few-cycle infrared laser pulses, we investigated the excitation and ionization of inner-shell electrons through laser-induced electron re-collision with the original parent ions and measured the dependence of the emitted x-ray spectra on the intensity and ellipticity of the driving laser. These directly re-colliding electrons can be used as the initiating pump step in pump/probe experiments for studying core-hole dynamics at their natural temporal scale. In our experiment we found that the dependence of the x-ray emission spectrum on the laser intensity and polarization state varies distinctly for the two kinds of atomic systems. Relying on our data and numerical simulations, we explain this behavior by the presence of different excitation mechanisms that are contributing in different ratios to the respective overall x-ray emission yields. Direct re-collision excitation competes with indirect collisions with neighboring atoms by electrons having "drifted away" from the original parent ion. (C) 2020 Optical Society of America under the terms of the OSA Open Access Publishing Agreement 
650 4 |a Fizikai tudományok 
700 0 1 |a Zeng Zhinan  |e aut 
700 0 1 |a Komm Pavel  |e aut 
700 0 1 |a Zheng Yinghui  |e aut 
700 0 1 |a Helml Wolfram  |e aut 
700 0 1 |a Xie Xinhua  |e aut 
700 0 1 |a Filus Zoltán  |e aut 
700 0 1 |a Dumergue Mathieu  |e aut 
700 0 1 |a Flender Roland  |e aut 
700 0 1 |a Kurucz Máté  |e aut 
700 0 1 |a Haizer Ludovit  |e aut 
700 0 1 |a Kiss Bálint  |e aut 
700 0 1 |a Kahaly Subhendu  |e aut 
700 0 1 |a Li Ruxin  |e aut 
700 0 1 |a Marcus Gilad  |e aut 
856 4 0 |u http://publicatio.bibl.u-szeged.hu/26944/1/31733452.pdf  |z Dokumentum-elérés